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Followed by Journey, she appeared in a string of successful films like Seethamma Vakitlo Sirimalle Chettu, Balupu, Masala, Geethanjali and Dictator, which made her one of the leading actresses in Telugu.
She also received two Nandi awards for best actress for her performances in the films Seethamma Vakitlo Sirimalle Chettu &Geethanjali.
The director also began two other films with Anjali, Valiba Desam and En Kanavu Thaanadi, though those also failed to materialise.
During one of her modelling assignments, she was spotted by director Siva Nageswara Rao, who offered her a starring role in his Telugu thriller film Photo (2006).
Anjali won critical praise for her portrayal of Anandhi, the childhood friend and love interest of a young teacher-turned-psychopath (enacted by Jeeva).
A Behindwoods critic wrote that she was "a delight to watch and spellbinds the viewer with her beautiful fresh look and her performance", She appeared in two films in 2008; Honganasu, her first Kannada project and Aayudham Seivom in Tamil.
She was labelled 'traditional' after Gokulamlo Seetha.
She also worked in the Bollywood Hindi movies Rangbaaz (1996), Suraj (1997) and Jodidar (1997) with superstar Mithun Chakraborty.
Meanwhile, she was cast by director A R Murugadoss to perform a lead role in his maiden production Engeyum Eppodhum alongside Jai, Sharvanand and Ananya, directed by his assistant M Saravanan.s Pavithra Srinivasan cited it was her "who clearly walks away with the honours", adding that "the extent of her feelings emerges only at the end, and carries you away" and calling it a "noteworthy performance".
In 2013, she starred in the Telugu multi-starrer Seethamma Vakitlo Sirimalle Chettu along with Venkatesh, Mahesh Babu and Samantha.
Her clothes, hair and makeup have all been changed to suit her character—that of a very confident and attractive Mumbai-based journalist".
In 2014, she appeared in a women centric horror film titled Geethanjali for the first time in her career.